After playing around with the Music Store in iTunes4, I thought it would be nice to be able to browse my library to be sure I wasn't buying something I already own. I created a smart playlist called "Whole Library" with just one condition - size is greater than 0 MB with Live Updating checked. Then I can double click on this playlist to bring it up in a separate window and can do searches, or browse (Edit -> Show Browser) while shopping in the main iTunes window.
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